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Learn how to stop automatic syncing for all iPods, iPhones, and iPads.
1. Open iTunes on your iPhone
2. Select iTunes then Preferences (if you are on a Mac), or select Edit > Preferences (if you are on a PC)
3. Click to open Devices
4. Select “Prevent iPods, iPhones, and iPads from syncing automatically”.
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If you tick in this checkbox, iPhone will not sync, even when “Open iTunes when this iPhone is connected” is enabled.
Read: iPhone 4: How to Prevent Automatic Syncing for all iPods, iPhones, and iPads